Reference: E.J. Garboczi and D.P. Bentz, Journal of Materials Science 27, 2083-2092 (1992).

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Computer Simulation of the Diffusivity of Cement-Based Materials

E.J. Garboczi and D.P. Bentz
National Institute of Standards and Technology
Building Materials Division, 226/B348
Gaithersburg, Maryland 20899


Abstract

A digital-image-based model of the microstructure of cement paste, coupled with exact transport algorithms, are used to study the diffusivity of portland cement paste. The principal variables considered are water:cement ratio, degree of cement hydration, and capillary porosity. Computational methods are described, and diffusivity results are presented, which are found to agree within experimental error with the available experimental measurements. Model cement pastes prepared with different water:cement ratios, and having different degrees of hydration, are found to have diffusivities that lie on a single master curve when plotted as a function of capillary porosity. Concepts from percolation theory are used to quantitatively explain the dependence of diffusivity on capillary porosity. The effect of silica fume addition on diffusivity is also examined.

1. Introduction
2. Digital-Image-Based Microstructural Model
3. Percolation Properties of the Pore Space
4. Computational Methods
5. Diffusivity Results
6. Cement Paste Diffusivity Dependence on Pore Structure
7. Summary
References


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