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Surface Area Calculations.

To understand the increase in wavelength () and the decrease in the growth rate of the instability in the moderately confined regime, we turn to a simple (in principle) calculation of the surface area of a thread when the fluctuation is no longer axisymmetric but somewhat flattened as depicted in Figure 1. The simplifying assumption behind this calculation is that the principal effect of the complex hydrodynamic interactions between the thread and the confining wall is to cause a fluctuation that is nonaxisymmetric. The cross section of the thread is no longer circular, but rather ellipsoidal at the bulges. We consider the nonaxisymmetry to be a fixed feature of the instability and then calculate the critical wavenumber Xc.

We assume that the surface equation of our nonaxisymmetric sinusoidal thread is expressed by the following equation:


where


Equation 6 describes that the cross section at the maximum perimeter (z = ) is an ellipse with a major axis of r' + and a minor axis of r' + , as depicted in Figure 1.

Here, we assume that the amplitude growth toward the wall, , is


and f can be defined as a degree of flattening. Equation 9 is supported by the observation described in the last section that / is approximately constant during the growth of the instability. Next, we calculate the surface area of the nonaxisymmetric sinusoidal thread as a function of the dimensionless wavenumber, the degree of flattening, and the relative amplitude.

Utilizing volume conservation of the thread during nonaxisymmetric growth and assuming that the cross section at the neck is circular (r' - = r' - ) (as found in the simulations), we obtain the following relations:




Then surface area of the thread per is as follows:25


Equation 12 cannot be integrated analytically. However, its first and second derivative with respect to at 0 can be obtained analytically. The results are as follows:




Equation 14 is a necessary condition for the distortion growth.

In Figure 12, we present the surface area of the sinusoidal thread divided by that of initial thread vs the amplitude at two different values of f. For the axisymmetric case of f = 1 (Figure 12A), we plot the normalized surface area for three different values of X. We see that only distortions with X < 1 cause a decrease in surface area, as discussed previously, i.e., Xc(f=1) = 1. In Figure 12B, making f < 1 captures the nonaxisymmetric growth of the thread, and we see its effect on surface area is different. We find that the critical wavenumber is shifted. For f = 0.5, we now have Xc (f=0.5) = 0.687. We present a plot of the critical wavenumber (2R0/c) vs f in Figure 13. The critical wavenumber decreases with decreasing f. Thus, the wavelength increases as a result of confinement in a manner similar to the experiment. It is interesting that the critical wavenumber becomes zero below a certain value of f (0.36). That may explain our experimental result that the thread placed between a gap whose size slightly larger than the thread diameter does not show the distortion growth at all. The dominant wavenumber, Xm, at which the amplitude grows fastest will also decrease as the critical wavenumber decreases. Experimentally, we observe Xm rather than Xc.

Figure 12. Normalized surface area of a nonaxisymmetric sinusoidal cylinder as a function of relative amplitude. Numbers in each curve represent dimensionless wavenumbers. (a) f = 1, (b) f = 0.5.
Figure 13. Critical dimensionless wavenumber (D0/c) vs +/. c is a minimum wavelength, which allows the distortion growth.

Intuitively, we can understand the above result on the basis of eqs 4 and 5. The reduction of surface area upon the growth of a fluctuation occurs in an axisymmetric thread because the average radius (denoted by R' in Figure 1) of the thread must decrease in order to conserve volume. In the nonaxisymmetric case, this decrease in the average radius is less, and so the increase in surface area due to the contour length increase becomes dominant. Note that f cannot be predicted from the present analysis for a given degree of confinement and viscosity ratio. Our primary goal in the surface area calculations is to show that forcing the growth to be nonaxisymmetric can cause the wavelength to increase and to reduce the driving force for breakup. We note that other choices for the shape of the nonaxisymmetric thread are possible other than that described. For example, we also considered a shape wherein the inflection point was circular and both the bulges and necks were elliptical. This too produced a similar result with a slightly smaller value of f where the critical wavenumber becomes zero. While our choices of axisymmetric growth is consistent with experiment and simulation, a more rigorous approach would utilize a calculus of variations coupled with knowledge of the initial grow rates in the parallel and perpendicular directions.


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